So, we'll see what you think, but Baccano will probably have a real confusing effect on you due to its form of story telling. I would actually suggest you move on straight to another short show, FLCL, just to see it as a piece of art. Then, since you'll be sufficiently weirded out by then, move to something more standard. Like Full Metal Alchemist or Ghost in the Shell.
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"I can already feel my Dumey Lust kicking in." -MistBiomeZ