Yeah I think if we're including Netflix shows my ranking of villains is Kilgrave 1, Kingpin 1a lol. Those guys both absolutely crushed their roles
As far as just the movies/Disney+ series go though Vulture's my fave, followed by I guess Thanos even though it's a boring answer but he IS really good
but Thanos is never as threatening or scary as Michael Keaton in the car. holy s h i t